Pump−probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL - Université de Lorraine
Journal Articles Journal of Synchrotron Radiation Year : 2017

Pump−probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL

Mathieu G Silly
Marie Agnès Tordeux
  • Function : Author
Debora Pierucci
Nathan Beaulieu
Christian Chauvet
  • Function : Author
Federico Pressacco
Fausto Sirotti
Horia Popescu
  • Function : Author
Victor Lopez-Flores
  • Function : Author
Marina Tortarolo
  • Function : Author
Maurizio Sacchi
Nicolas Jaouen
Philippe Hollander
  • Function : Author
Jean Paul Ricaud
  • Function : Author
Nicolas Bergeard
  • Function : Author
  • PersonId : 917019
Bharati Tudu
  • Function : Author
Renaud Delaunay
Jan Lüning
Grégory Malinowski
Michel Hehn
Cédric Baumier
  • Function : Author
Franck Fortuna
Damjan Krizmancic
  • Function : Author
Luigi Stebel
  • Function : Author
Rudi Sergo
  • Function : Author
Giuseppe Cautero
  • Function : Author

Abstract

The SOLEIL synchrotron radiation source is regularly operated in special filling modes dedicated to pump–probe experiments. Among others, the low-mode operation is characterized by shorter pulse duration and represents the natural bridge between 50 ps synchrotron pulses and femtosecond experiments. Here, the capabilities in low-mode of the experimental setups developed at the TEMPO beamline to perform pump–probe experiments with soft X-rays based on photoelectron or photon detection are presented. A 282 kHz repetition-rate femtosecond laser is synchronized with the synchrotron radiation time structure to induce fast electronic and/or magnetic excitations. Detection is performed using a two-dimensional space resolution plus time resolution detector based on microchannel plates equipped with a delay line. Results of time-resolved photoelectron spectroscopy, circular dichroism and magnetic scattering experiments are reported, and their respective advantages and limitations in the framework of high-time-resolution pump–probe experiments compared and discussed.
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Dates and versions

hal-01624336 , version 1 (26-10-2017)

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Mathieu G Silly, Tom Ferté, Marie Agnès Tordeux, Debora Pierucci, Nathan Beaulieu, et al.. Pump−probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL. Journal of Synchrotron Radiation, 2017, 24 (4), pp.886 - 897. ⟨10.1107/S1600577517007913⟩. ⟨hal-01624336⟩
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